Discovery Learning accelerates battery design evaluation

Fast and reliable validation of novel designs in complex physical systems such as batteries is critical to accelerating technological innovation. However, battery research and development remain bottlenecked by the prohibitively high time and energy costs required to evaluate numerous new design candidates, particularly in battery prototyping and life testing. Despite recent progress in data-driven battery lifetime prediction, existing methods require labeled data of target designs to improve accuracy and cannot make reliable predictions until after prototyping, thus falling far short of the efficiency needed to enable rapid feedback for battery design. Here, we introduce Discovery Learning (DL), a scientific machine-learning paradigm that integrates active learning, physics-guided learning, and zero-shot learning into a human-like reasoning loop, drawing inspiration from learning theories in educational psychology. DL can learn from historical battery designs and actively reduce the need for prototyping, thus enabling rapid lifetime evaluation for unobserved material-design combinations without requiring additional data labeling. To test DL, we present 123 industrial-grade large-format lithium-ion pouch cells, spanning eight material-design combinations and diverse cycling protocols. Trained solely on public datasets of small-capacity cylindrical cells, DL achieves 7.2% test error in predicting the average cycle life under unknown device variability. This results in savings of 98% in time and 95% in energy compared to industrial practices. This work highlights the potential of uncovering insights from historical designs to inform and accelerate the development of next-generation battery technologies. DL represents a key advance toward efficient data-driven modeling and helps realize the promise of machine learning for accelerating scientific discovery and engineering innovation.

Enhanced Battery Capacity Estimation in Data-Limited Scenarios through Swarm Learning

Data-driven methods have shown potential in electric-vehicle battery management tasks such as capacity estimation, but their deployment is bottlenecked by poor performance in data-limited scenarios. Sharing battery data among algorithm developers can enable accurate and generalizable data-driven models. However, an effective battery management framework that simultaneously ensures data privacy and fault tolerance is still lacking. This paper proposes a swarm battery management system that unites a decentralized swarm learning (SL) framework and credibility weight-based model merging mechanism to enhance battery capacity estimation in data-limited scenarios while ensuring data privacy and security. The effectiveness of the SL framework is validated on a dataset comprising 66 commercial LiNiCoAlO2 cells cycled under various operating conditions. Specifically, the capacity estimation performance is validated in four cases, including data-balanced, volume-biased, feature-biased, and quality-biased scenarios. Our results show that SL can enhance the estimation accuracy in all data-limited cases and achieve a similar level of accuracy with central learning where large amounts of data are available.