Many genus-0 surface mapping tasks such as landmark alignment, feature matching, and image-driven registration, can be reduced (via an initial spherical conformal map) to optimizing a spherical self-homeomorphism with controlled distortion. However, existing works lack efficient mechanisms to control the geometric distortion of the resulting mapping. To resolve this issue, we formulate this as a Beltrami-space optimization problem, where the angle distortion is encoded explicitly by the Beltrami differential and bijectivity can be enforced through the constraint $\|μ\|_{\infty}<1$. To make this practical on the sphere, we introduce the Spherical Beltrami Differential (SBD), a two-chart representation of quasiconformal self-maps of the unit sphere $\mathbb{S}^2$, together with cross-chart consistency conditions that yield a globally bijective spherical deformation (up to conformal automorphisms). Building on the Spectral Beltrami Network, we develop BOOST, a differentiable optimization framework that updates two Beltrami fields to minimize task-driven losses while regularizing distortion and enforcing consistency along the seam. Experiments on large-deformation landmark matching and intensity-based spherical registration demonstrate improved task performance meanwhile maintaining controlled distortion and robust bijective behavior. We also apply the method to cortical surface registration by aligning sulcal landmarks and matching cortical sulcal depth, achieving comparative or better registration performance without sacrificing geometric validity.